Juliet Stevenson, who played Desiree in the NYCO production opposite Jeremy Irons, was perfect. I'd love to see her do the role on Broadway, but I don't think she's enough of a "name" to be seriously considered. Kate Burton would also be a good choice, as would Elaine Paige.
How about Vanessa Redgrave for Mme. Armfeldt?
"You travel alone because other people are only there to remind you how much that hook hurts that we all bit down on. Wait for that one day we can bite free and get back out there in space where we belong, sail back over water, over skies, into space, the hook finally out of our mouths and we wander back out there in space spawning to other planets never to return hurrah to earth and we'll look back and can't even see these lives here anymore. Only the taste of blood to remind us we ever existed. The earth is small. We're gone. We're dead. We're safe."
-John Guare, Landscape of the Body